Also known as state transfer · state-to-state · entangled state preparation · cooling
State preparation drives a quantum system from a known initial state into a target state: a superposition, an
entangled state of many qubits, the ground state of a many-body Hamiltonian, a Fock or cat state of an oscillator.
State transfer moves an unknown state from one place to another, along a chain or between distant nodes. These
were the first problems of quantum control, in the steering of molecular wave packets to select chemical products
[1, 2, 3]. They remain the most common ones outside gate
design.
The problem
For pure states, the objective is the overlap \(F = |\langle\psi_\mathrm{target}|\psi(T)\rangle|^2\). It involves one
state rather than a full unitary, so it is cheaper to compute and needs fewer control resources. Its
landscape is generically free of traps when the system is controllable. For mixed or open
systems, the objective becomes a distance between density matrices or the expectation of a projector. See
Problem formulation & figures of merit. The minimal duration is set by the speed limit, and an optimizer scanning the duration
finds it as the time below which the target can no longer be reached [4].
Routes to a target state
Adiabatic following. Slowly changing the Hamiltonian keeps the system in an eigenstate that connects the
initial and target states. STIRAP and rapid adiabatic passage transfer population completely and robustly
[5, 6]. Adiabatic quantum computation prepares ground states of problem
Hamiltonians the same way [7]. See Adiabatic passage.
Shortcuts. Shortcuts to adiabaticity reach the same final state in a finite time [8], for example
cooling atoms in harmonic traps fast and without final excitation [9]. See
Shortcuts to adiabaticity.
Optimal control. Numerical optimization handles the cases without analytic solutions, from single qubits to
many-body states [10, 11]. See GRAPE, CRAB & dCRAB and Many-body optimal control.
Constructive sequences. For an oscillator coupled to a qubit, any state can be built step by step
[12], as done for arbitrary superpositions of photon numbers [13]. See
Bosonic & continuous-variable control.
Circuits. Entangling gates build GHZ states. In 14 trapped ions, their coherence decayed with the square of the
number of qubits, as expected for correlated phase noise [14].
Measurement and feedback. Real-time feedback prepared and stabilized photon-number states in a cavity
[17]. See Measurement-based feedback.
State transfer
Along spin chains. Even an unmodulated Heisenberg chain transmits a qubit with better-than-classical fidelity
over tens of spins [18]. With engineered but fixed couplings, the transfer is perfect over any length
of chain [19]. With time-dependent control, the transfer can run at the speed limit
[20], and control at one end of the chain can be enough [21].
Between distant nodes. In a quantum network, a laser pulse can map an atom’s state onto a time-symmetric photon
that a second atom absorbs with unit probability [22]. The microwave version transferred states
deterministically between superconducting qubits on separate chips [23].
Cooling and initialization
Preparing a pure state from a thermal one requires removing entropy, so it needs dissipation or measurement. Optimal
control has been used to design laser cooling of internal molecular degrees of freedom [24]. The
third law limits how fast this can go: for general cooling processes, the attainable temperature scales as an inverse
power of the cooling time [25]. Fast, unconditional reset of qubits is part of
Control for quantum error correction[26]; see also Control in quantum thermodynamics.
In experiments
Cold atoms. Closed-loop optimization sped up atom loading into optical lattices and the crossing of the
superfluid–Mott-insulator transition more than threefold [27]. With condensates in optical lattices,
both a protocol at the speed limit and a robust superadiabatic (transitionless) protocol were realized
[28]. See Ultracold atoms & BECs.
Citizen science. In a game based on moving atoms with optical tweezers, players found good solutions in
regimes where purely numerical optimization struggled [29].
Limitations
Verifying a large entangled state is hard: tomography scales exponentially, and witnesses or fidelity estimates
replace it.
A state-to-state solution works only for the initial state it was designed for, while a gate works for all
inputs. Errors in the initial state propagate.
Many optimal solutions exist for the same target, and the choice between them should be based on robustness rather
than nominal fidelity alone.
Key papers
David J. Tannor and Stuart A. RiceControl of selectivity of chemical reaction via control of wave packet evolutionThe Journal of Chemical Physics83, 5013-5018 (1985)doi
Steering molecular wave packets with timed pulses to select the outcome of a chemical reaction — an origin of state-to-state control.
K. Bergmann, H. Theuer and B. W. ShoreCoherent population transfer among quantum states of atoms and moleculesRev. Mod. Phys.70, 1003-1025 (1998)doi
Review of STIRAP and related adiabatic methods for complete, robust population transfer.
T. Caneva, M. Murphy, T. Calarco, R. Fazio, S. Montangero, et al.Optimal Control at the Quantum Speed LimitPhys. Rev. Lett.103, 240501 (2009)doi
Optimal control reaches the target state exactly down to a minimal time that coincides with the quantum speed limit.
Matthias Christandl, Nilanjana Datta, Artur Ekert and Andrew J. LandahlPerfect State Transfer in Quantum Spin NetworksPhys. Rev. Lett.92, 187902 (2004)doi
Spin networks with fixed, engineered couplings that transfer any state perfectly, without switching.
J. I. Cirac, P. Zoller, H. J. Kimble and H. MabuchiQuantum State Transfer and Entanglement Distribution among Distant Nodes in a Quantum NetworkPhys. Rev. Lett.78, 3221-3224 (1997)doi
Transfer between distant atoms by shaping the emitted photon so that it is absorbed with unit probability.
B. Kraus, H. P. Büchler, S. Diehl, A. Kantian, A. Micheli and P. ZollerPreparation of entangled states by quantum Markov processesPhys. Rev. A78, 042307 (2008)doi
Any pure entangled state can be prepared as the unique steady state of an engineered dissipative process.
References
David J. Tannor and Stuart A. RiceControl of selectivity of chemical reaction via control of wave packet evolutionThe Journal of Chemical Physics83, 5013-5018 (1985)doi
R. Kosloff, S.A. Rice, P. Gaspard, S. Tersigni and D.J. TannorWavepacket dancing: Achieving chemical selectivity by shaping light pulsesChemical Physics139, 201-220 (1989)doi
Herschel Rabitz, Regina de Vivie-Riedle, Marcus Motzkus and Karl KompaWhither the Future of Controlling Quantum Phenomena?Science288, 824-828 (2000)doi
T. Caneva, M. Murphy, T. Calarco, R. Fazio, S. Montangero, et al.Optimal Control at the Quantum Speed LimitPhys. Rev. Lett.103, 240501 (2009)doi
K. Bergmann, H. Theuer and B. W. ShoreCoherent population transfer among quantum states of atoms and moleculesRev. Mod. Phys.70, 1003-1025 (1998)doi
Nikolay V. Vitanov, Andon A. Rangelov, Bruce W. Shore and Klaas BergmannStimulated Raman adiabatic passage in physics, chemistry, and beyondRev. Mod. Phys.89, 015006 (2017)doi
Tameem Albash and Daniel A. LidarAdiabatic quantum computationRev. Mod. Phys.90, 015002 (2018)doi
D. Guéry-Odelin, A. Ruschhaupt, A. Kiely, E. Torrontegui, S. Martínez-Garaot and J. G. MugaShortcuts to adiabaticity: Concepts, methods, and applicationsRev. Mod. Phys.91, 045001 (2019)doi
Xi Chen, A. Ruschhaupt, S. Schmidt, A. del Campo, D. Guéry-Odelin and J. G. MugaFast Optimal Frictionless Atom Cooling in Harmonic Traps: Shortcut to AdiabaticityPhys. Rev. Lett.104, 063002 (2010)doi
Patrick Doria, Tommaso Calarco and Simone MontangeroOptimal Control Technique for Many-Body Quantum DynamicsPhys. Rev. Lett.106, 190501 (2011)doi
A. Omran, H. Levine, A. Keesling, G. Semeghini, T. T. Wang, et al.Generation and manipulation of Schrödinger cat states in Rydberg atom arraysScience365, 570-574 (2019)doi
C. K. Law and J. H. EberlyArbitrary Control of a Quantum Electromagnetic FieldPhys. Rev. Lett.76, 1055-1058 (1996)doi
Max Hofheinz, H. Wang, M. Ansmann, Radoslaw C. Bialczak, Erik Lucero, et al.Synthesizing arbitrary quantum states in a superconducting resonatorNature459, 546-549 (2009)doi
Thomas Monz, Philipp Schindler, Julio T. Barreiro, Michael Chwalla, Daniel Nigg, et al.14-Qubit Entanglement: Creation and CoherencePhys. Rev. Lett.106, 130506 (2011)doi
B. Kraus, H. P. Büchler, S. Diehl, A. Kantian, A. Micheli and P. ZollerPreparation of entangled states by quantum Markov processesPhys. Rev. A78, 042307 (2008)doi
Frank Verstraete, Michael M. Wolf and J. Ignacio CiracQuantum computation and quantum-state engineering driven by dissipationNature Phys5, 633-636 (2009)doi
Clément Sayrin, Igor Dotsenko, Xingxing Zhou, Bruno Peaudecerf, Théo Rybarczyk, et al.Real-time quantum feedback prepares and stabilizes photon number statesNature477, 73-77 (2011)doi
Sougato BoseQuantum Communication through an Unmodulated Spin ChainPhys. Rev. Lett.91, 207901 (2003)doi
Matthias Christandl, Nilanjana Datta, Artur Ekert and Andrew J. LandahlPerfect State Transfer in Quantum Spin NetworksPhys. Rev. Lett.92, 187902 (2004)doi
Michael Murphy, Simone Montangero, Vittorio Giovannetti and Tommaso CalarcoCommunication at the quantum speed limit along a spin chainPhys. Rev. A82, 022318 (2010)doi
Daniel Burgarth, Sougato Bose, Christoph Bruder and Vittorio GiovannettiLocal controllability of quantum networksPhys. Rev. A79, 060305 (2009)doi
J. I. Cirac, P. Zoller, H. J. Kimble and H. MabuchiQuantum State Transfer and Entanglement Distribution among Distant Nodes in a Quantum NetworkPhys. Rev. Lett.78, 3221-3224 (1997)doi
P. Kurpiers, P. Magnard, T. Walter, B. Royer, M. Pechal, et al.Deterministic quantum state transfer and remote entanglement using microwave photonsNature558, 264-267 (2018)doi
Allon Bartana, Ronnie Kosloff and David J. TannorLaser cooling of internal degrees of freedom. IIThe Journal of Chemical Physics106, 1435-1448 (1997)doi
Lluís Masanes and Jonathan OppenheimA general derivation and quantification of the third law of thermodynamicsNat Commun8, 14538 (2017)doi
P. Magnard, P. Kurpiers, B. Royer, T. Walter, J.-C. Besse, et al.Fast and Unconditional All-Microwave Reset of a Superconducting QubitPhys. Rev. Lett.121, 060502 (2018)doi
S. Rosi, A. Bernard, N. Fabbri, L. Fallani, C. Fort, et al.Fast closed-loop optimal control of ultracold atoms in an optical latticePhys. Rev. A88, 021601 (2013)doi
Mark G. Bason, Matthieu Viteau, Nicola Malossi, Paul Huillery, Ennio Arimondo, et al.High-fidelity quantum drivingNature Phys8, 147-152 (2012)doi
Jens Jakob W. H. Sørensen, Mads Kock Pedersen, Michael Munch, Pinja Haikka, Jesper Halkjær Jensen, et al.Exploring the quantum speed limit with computer gamesNature532, 210-213 (2016)doi
Recent papers
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Programmable preparation of entangled quantum states is a central requirement for scalable quantum information processing, quantum networking and photonic quantum computing. Topological photonic platforms offer an attractive route towards robust quantum-state generation by encoding information in symmetry- protected optical modes, yet the generated entangled states are typically dictated by the lattice geometry and therefore lack programmability. Here we demonstrate programmable preparation of topological entangled states by inverse engineering the nonlinear optical pump profile of an integrated photonic lattice. Our approach enables deterministic control over both the dimensionality and modal structure of the generated entangled state while preserving its topological character. We experimentally realize silicon photonic topological superlattices in which the nonlinear generation pathway itself becomes programmable via tailored excitations. The superlattices host a multiband manifold of co localized topological interface modes, while coherently controlled inputs synthesize pump superpositions within this protected basis. We showcase this principle by selectively addressing topological biphoton eigenstates, steering correlations to produce a desired target state in a high-dimensional Hilbert space, and inverse-designing pump states that generate targeted Schmidt dimensionalities. Site-resolved two-photon correlation measurements remain reproducible across nominally identical fabricated devices, demonstrating robustness to realistic nanofabrication-induced disorder. Programmable preparation of topological entangled states establishes a pathway towards exploiting topological photonic modes as application-specific quantum resources, enabling tailored input states for high-dimensional quantum communication, quantum networking and photonic quantum computing.
Preparing quantum states in bosonic qudits with SNAP--Displacement sequences requires both optimizing the gate parameters and deciding which Fock levels should be controlled by each SNAP gate. A fully parameterized ansatz assigns an independent phase to every Fock level in every gate, leading to a number of phases that grows steeply. This constitutes a problem for short to medium term systems as controlling many phases requires complex control pulses which are subject to increased control errors. Previous work reduced this cost by restricting the trainable phases to predefined sparse patterns, such as a diagonal or a grid, which however may not be optimal for a specific target state. In this work, we address this limitation by introducing a method that learns which phases are needed together with their values, using a differentiable mask. A sparsity penalty encourages the removal of unnecessary phases, while temperature annealing gradually turns the masks into binary decisions. We compare the proposed method with fully parameterized and predefined sparse ansatzes on Fourier and Haar-random target states. The evaluation considers both the minimum number of phases required to reach different infidelity thresholds and the overall trade-off between fidelity and phases required, measured through Pareto frontiers and hypervolume. The results show that learning the location of the phases together with their values provides competitive or improved fidelity--resource trade-offs, although the advantage depends on the target state and qudit dimension.
Multimode mechanical resonators offer a large set of densely packed, long-lived bosonic modes within a single compact device, making them attractive for quantum simulation, quantum information processing, and quantum-enhanced sensing. Many such applications rely on multipartite entanglement, yet deterministic mechanical entanglement has so far been largely limited to pairs of modes. Here we demonstrate the deterministic and programmable preparation of multipartite entangled states among the phonon modes of a high-overtone bulk acoustic wave resonator coupled to a superconducting transmon qubit. By sequentially applying optimal-control-engineered isometries between the qubit and successive modes, we generate matrix product states of bond dimension two, including $W$, Greenberger-Horne-Zeilinger (GHZ), and cluster states. We fully characterize these states via quantum state tomography and certify genuine multipartite entanglement among up to four modes. We further demonstrate correlated-noise sensing by exploiting the complementary decoherence responses of the stored $W$ and GHZ states, isolating inter-mode phase correlations from local decoherence and placing quantitative bounds on collective dephasing. Our results establish a scalable approach to preparing multipartite entangled states in mechanical systems, with promising applications in multiparameter sensing and tests of quantum mechanics with massive objects.
We describe an optimal-control strategy designed to accelerate the dissipative preparation of complex, highly entangled quantum many-body states. Analogous to optimal steering of isolated quantum systems, our scheme identifies control pulses that guide the evolution of open quantum systems along trajectories of instantaneous steady states while minimizing leakage resulting from non-adiabatic transitions. In many cases of interest, these control parameters can be derived analytically and without the need for computationally expensive numerical simulations of the full many-body master equation. We apply this technique for the preparation of bi- and multipartite entangled states in qubit systems coupled to a common photonic waveguide or a distributed squeezed reservoir. In both scenarios, our optimal-control strategy significantly outperforms the bare relaxation dynamics after a quench, reducing preparation times of near-maximally entangled states by orders of magnitude. This drastic speedup makes dissipative entanglement distribution protocols compatible with high-fidelity quantum information processing applications and illustrates more broadly the potential of leakage minimization for accelerating reservoir-engineering schemes.
Many-body entanglement in atomic ensembles offers the potential for enhanced sensing devices. Entanglement can be generated by interfacing atoms with a cavity. Traditional methods use effective two-level systems isolated from more complex atomic level structures. However, alternative strategies allow entanglement to be generated in atoms confined to a single hyperfine manifold. These strategies enable entanglement in ways fundamentally not available to two-level systems but feature extremely slow dynamics due to requiring strongly off-resonant laser fields. Here, I show that equivalent squeezing dynamics can be achieved much closer to resonance, offering entanglement generation over a hundred times faster than typical experiments. Furthermore, the Hamiltonian can be used to speed up the creation of maximally entangled states via adiabatic passage.