Also known as closed-loop optimization · in situ · adaptive feedback control · ad-HOC · hybrid optimal control · calibration
Even the best model of a quantum device is imperfect. Unknown couplings, pulse distortions and drifting parameters make
pulses optimized on a computer underperform on hardware. Closed-loop (or in situ) optimization removes the model
from the loop. An optimizer proposes a control, the experiment measures how well it works, and the result guides
the next proposal. Introduced in chemistry as learning control[1], it is now routine for calibrating
gates in quantum processors.
The loop
Propose controls \(u\) (often in a compact parametrization — a few amplitudes, phases, or CRAB
coefficients).
Run the experiment and estimate a figure of merit \(\hat J(u)\) — a state population, a randomized-benchmarking
fidelity, a sensing signal.
Update \(u\) with an optimizer that tolerates noisy estimates, and repeat.
The figure of merit is noisy, since every estimate comes from finitely many shots, and expensive, since every
evaluation costs experimental time. This shapes the choice of optimizer and of objective.
Gradient-free closed loops
The classic choice is a gradient-free method: genetic algorithms, Nelder–Mead or CMA-ES.
Chemistry. Feedback-optimized, phase-shaped femtosecond pulses steered the branching ratio of chemical reactions
[2]; see Molecules & chemical control.
Superconducting qubits. Nelder–Mead with randomized benchmarking as the objective tunes single- and two-qubit gates
and identifies crosstalk [3]. “Restless” measurements, which skip the wait for qubit relaxation,
speed up the tune-up tenfold, reaching 0.999 average Clifford fidelity in about a minute [4].
Optimizing every sample of the waveform in closed loop produced a 4.16 ns gate with 0.044 % leakage
[5].
Spins and atoms. Autonomous closed-loop calibration of NV-centre spin operations [6], online
optimization of ultracold-atom experiments with machine-learning surrogates [7], and remote
optimization involving citizen scientists [8].
Hybrid: model first, device second
Pure closed-loop optimization from scratch is slow. Ad-HOC first optimizes on a model with gradients, then refines
the near-optimal pulse on the device with a gradient-free search. In typical solid-state settings this improved gate
fidelities by an order of magnitude [9]. Starting from a good model-based guess, and optimizing only the
few parameters that matter, is the most common practical strategy.
Gradients from the device
Gradients can also be measured. In a hybrid quantum–classical scheme, the quantum system evaluates the fitness and its
gradient while a classical computer updates the controls. This was demonstrated on a seven-qubit NMR processor
[10]. Measured gradients (and finite differences) have been compared with open-loop optimization in a
solid-state two-qubit system [11]. A 12-qubit processor has been used to optimize its own control
sequence with measurement-based feedback, correcting unknown imperfections [12]. More generally, a
quantum simulator can learn its own gates in situ. This avoids both an accurate model and a classical computer more
powerful than the simulator, with evidence of polynomial scaling up to nine qubits [13].
Coping with noisy, expensive evaluations
Stochastic optimization. Algorithms built on direct fidelity estimation need only a constant number of
experiments per iteration, independent of the number of control parameters. They are robust to statistical and
technical noise [14].
Bayesian optimization builds a surrogate model of the landscape and chooses the most informative next
experiment. It finds optimal controls even with very few shots per setting, down to single-shot measurements
[15]; see Reinforcement & machine learning for control.
Cheap, sensitive objectives. Randomized benchmarking, restless measurements and error-amplifying sequences make
each evaluation fast and sensitive to small errors.
Closed loop versus model learning
Closed-loop optimization treats the device as a black box. The alternative is to learn a better model from data and
optimize on it (System identification for control). The two combine naturally: identify, optimize, verify, refine
[16]. Re-optimizing continuously over a short horizon leads to model-predictive control
(Lyapunov, tracking & model-predictive control).
Strengths and limitations
Strengths
Accounts for everything the model misses: distortions, crosstalk, unknown couplings.
Simple to set up on top of existing calibration routines.
Limitations
Every evaluation costs experimental time, and shot noise limits precision.
Scales poorly with the number of parameters unless gradients or surrogate models are used.
Results are specific to the device and can drift, so periodic re-calibration is needed.
Key papers
Richard S. Judson and Herschel RabitzTeaching lasers to control moleculesPhys. Rev. Lett.68, 1500-1503 (1992)doi
Proposes learning control. Let an algorithm "teach" the laser by optimizing directly on the experiment, without a model.
D. J. Egger and F. K. WilhelmAdaptive Hybrid Optimal Quantum Control for Imprecisely Characterized SystemsPhys. Rev. Lett.112, 240503 (2014)doi
Ad-HOC. Optimize on a model first, then refine on the device with a gradient-free method, combining the strengths of both.
J. Kelly, R. Barends, B. Campbell, Y. Chen, Z. Chen, et al.Optimal Quantum Control Using Randomized BenchmarkingPhys. Rev. Lett.112, 240504 (2014)doi
Closed-loop gate tuning on superconducting qubits with randomized benchmarking as the objective.
Jun Li, Xiaodong Yang, Xinhua Peng and Chang-Pu SunHybrid Quantum-Classical Approach to Quantum Optimal ControlPhys. Rev. Lett.118, 150503 (2017)doi
A hybrid scheme in which the quantum device itself evaluates the fidelity and its gradient for a classical optimizer.
Frédéric Sauvage and Florian MintertOptimal Quantum Control with Poor StatisticsPRX Quantum1, 020322 (2020)doi
Bayesian optimization that finds optimal controls even with large shot noise, down to single-shot measurements.
Software
QuOCS — optimal control suite designed to talk to experiments (dCRAB, Nelder–Mead, CMA-ES, gradients)
C3 — integrates open-loop optimization, closed-loop calibration and model learning
References
Richard S. Judson and Herschel RabitzTeaching lasers to control moleculesPhys. Rev. Lett.68, 1500-1503 (1992)doi
A. Assion, T. Baumert, M. Bergt, T. Brixner, B. Kiefer, et al.Control of Chemical Reactions by Feedback-Optimized Phase-Shaped Femtosecond Laser PulsesScience282, 919-922 (1998)doi
J. Kelly, R. Barends, B. Campbell, Y. Chen, Z. Chen, et al.Optimal Quantum Control Using Randomized BenchmarkingPhys. Rev. Lett.112, 240504 (2014)doi
M. A. Rol, C. C. Bultink, T. E. O’Brien, S. R. de Jong, L. S. Theis, et al.Restless Tuneup of High-Fidelity Qubit GatesPhys. Rev. Applied7, 041001 (2017)doi
M. Werninghaus, D. J. Egger, F. Roy, S. Machnes, F. K. Wilhelm and S. FilippLeakage reduction in fast superconducting qubit gates via optimal controlnpj Quantum Inf7, 14 (2021)doi
Florian Frank, Thomas Unden, Jonathan Zoller, Ressa S. Said, Tommaso Calarco, et al.Autonomous calibration of single spin qubit operationsnpj Quantum Inf3, 48 (2017)doi
P. B. Wigley, P. J. Everitt, A. van den Hengel, J. W. Bastian, M. A. Sooriyabandara, et al.Fast machine-learning online optimization of ultra-cold-atom experimentsSci Rep6, 25890 (2016)doi
Robert Heck, Oana Vuculescu, Jens Jakob Sørensen, Jonathan Zoller, Morten G. Andreasen, et al.Remote optimization of an ultracold atoms experiment by experts and citizen scientistsProc. Natl. Acad. Sci. U.S.A.115 (2018)doi
D. J. Egger and F. K. WilhelmAdaptive Hybrid Optimal Quantum Control for Imprecisely Characterized SystemsPhys. Rev. Lett.112, 240503 (2014)doi
Jun Li, Xiaodong Yang, Xinhua Peng and Chang-Pu SunHybrid Quantum-Classical Approach to Quantum Optimal ControlPhys. Rev. Lett.118, 150503 (2017)doi
Guanru Feng, Franklin H. Cho, Hemant Katiyar, Jun Li, Dawei Lu, et al.Gradient-based closed-loop quantum optimal control in a solid-state two-qubit systemPhys. Rev. A98, 052341 (2018)doi
Dawei Lu, Keren Li, Jun Li, Hemant Katiyar, Annie Jihyun Park, et al.Enhancing quantum control by bootstrapping a quantum processor of 12 qubitsnpj Quantum Inf3, 45 (2017)doi
Benjamin Dive, Alexander Pitchford, Florian Mintert and Daniel BurgarthIn situ upgrade of quantum simulators to universal computersQuantum2, 80 (2018)doi
Christopher Ferrie and Osama MoussaRobust and efficient in situ quantum controlPhys. Rev. A91, 052306 (2015)doi
Frédéric Sauvage and Florian MintertOptimal Quantum Control with Poor StatisticsPRX Quantum1, 020322 (2020)doi
Nicolas Wittler, Federico Roy, Kevin Pack, Max Werninghaus, Anurag Saha Roy, et al.Integrated Tool Set for Control, Calibration, and Characterization of Quantum Devices Applied to Superconducting QubitsPhys. Rev. Applied15, 034080 (2021)doi
Recent papers
119 tracked papers since 2000 are classified
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Multi-tenant quantum processors expose a pulse-level attack surface in which coherent crosstalk can mimic benign calibration drift at matched average gate infidelity. We present a structural verification and detection framework based on the residual Pauli transfer matrix (PTM). We prove that products of local unital, trace-preserving channels cannot mix weight-1 and weight-2 Pauli operators, even under coherent drift of arbitrary strength or axis. Building on established PTM-to-Hamiltonian relations, we prove that, for any specified qubit pair in an arbitrarily large system, the first-order map from its nine interaction coefficients to the antisymmetric cross-weight feature is an isometry up to scale. Thus, every interaction direction is locally observable near the identity. We also exhibit cancellation of this feature under large local rotations and prove that the full cross-weight norm is invariant under local unitary composition, providing a structural countermeasure. For calibrated small local rotations, shared randomized-Pauli measurements support periodic verification using the evaluated antisymmetric detector. In simulation, $16{,}384$ randomized settings yield a detection threshold of $λ_{\min}\approx0.13$ at a $5\%$ calibrated false-positive target, with approximately $M^{-1/2}$ scaling in the number of settings $M$. Further experiments characterize detection under relaxation, depolarization, native ZZ fluctuations, and time-dependent pulse dynamics. Finally, an FRQI encoding with Pauli-graph quantum Hadamard edge detection reproduces the classical structural edge score to numerical precision.
Error-correction records can reveal noise yet supply the information needed for control too slowly. In a surface code under Gaussian dephasing, encoded calibration learns a correlation that reverses the preferred control mainly through rare events. A product probe exposes it more often through the same checks, reducing ideal-record sample complexity from inverse-square to inverse-linear in phase variance. Counting both calibration and execution costs, we show that this gain can repay probe overhead and enable protected tasks within budgets that exclude encoded calibration.
Quantum sensing increasingly demands materials combining room-temperature optical spin addressability and coherent control with rapid, accessible fabrication. Yet semiconductor platforms require costly materials and specialized processing, while molecular systems often depend on bespoke synthesis or involved crystal growth. Here we apply microspacing in-air sublimation (MAS) to rapidly fabricate quantum-sensing materials within minutes. Microgram quantities of commercially available precursors crystallize on glass, in air and without vacuum or inert-gas handling. Monitored in situ, growth yields optically clear, stoichiometric single crystals of excellent quality, including plates and needles with intrinsic optical waveguiding. Donor-acceptor charge-transfer co-crystals pairing anthracene or biphenyl with tetracyanobenzene, together with localized-exciton pentacene:pentacenequinone (P:PQ), exhibit room-temperature optically detected magnetic resonance (ODMR). Charge-transfer ODMR resonances reach linewidths below $4\mathrm{MHz}$, consistent with motional narrowing of mobile triplet excitons, while P:PQ supports coherent ensemble spin control with $T_2=0.56μ\mathrm{s}$. Functionality across chemically and electronically distinct pairs establishes MAS as an accessible screen for molecular quantum-sensing materials, connecting molecular crystal engineering with low-cost, chemically tunable thin triplet-spin layers and waveguiding sensor geometries for quantum sensing and microscopy.
We propose and demonstrate gates between two superconducting qubits based on quantum interference of consecutive Landau-Zener (LZ) transitions. This gate mechanism bridges between baseband and parametric two-qubit control, enabling in situ tuning of the control frequency across a continuous interval up to hundreds of MHz. Another advantage compared to dispersive couplers is that the speed of the LZ gate is on the order of the full coupling strength. We experimentally demonstrate the gate on two platforms, a modular chiplet architecture of coupled generalized flux qubits, and on a monolithic transmon architecture. The combination of tunability and gate speed establishes the LZ gate as a unique tool for multiplexing control pulses and interconnecting superconducting chiplet architectures.
We study measurement-based feedback control of a damped harmonic oscillator, motivated by optomechanical and interferometric position measurements, in which feedback is synthesized from a displacement measurement. For a band-limited derivative controller, the loop shapes the mechanical susceptibility and reinjects measurement noise, creating a tradeoff between stabilization and noise amplification. We present a compact classical formulation that isolates this tradeoff in the closed-loop displacement spectrum and identifies the parameters governing resonance suppression versus noise-driven actuation. We then extend the same topology to a quantum-limited position detector, enforcing the imprecision-backaction constraint and introducing finite measurement bandwidth that regularizes high-frequency noise reinjection and adds phase lag in the feedback path. In the high-$Q$ regime we obtain an analytic design rule for the optimal feedback gain at fixed controller and measurement bandwidths and compare it with full-spectrum calculations. The comparison shows that a high mechanical quality factor alone does not guarantee quantitative agreement: the accuracy of the near-resonant approximation depends strongly on the controller and measurement bandwidths. Because finite measurement bandwidth changes both the magnitude and phase of the feedback loop, the analysis separates the near-resonant damping contribution from imprecision-noise reinjection and shows that positive near-resonant feedback damping requires the product of the controller cutoff and measurement bandwidth to exceed the square of the mechanical resonance frequency. Finally, we present a dimensionless map of the gain-optimized high-$Q$ occupation and compare its predictions with full-spectrum optimization. All analytical gains evaluated in this map satisfy the full closed-loop stability criterion for these parameters.