CAGE team
Inria Paris and Sorbonne Université (Laboratoire Jacques-Louis Lions), Paris, France
- Website
- www.ljll.fr/boscain/
- Tracked papers
- 22 (2003–2026)
Topics
The most frequent field-map topics among the PIs' tracked papers.
Recent papers
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Local controllability of heralded quantum linear optics
Abstract
Photonic linear optical networks provide a versatile platform for quantum information processing and quantum state engineering. However, the set of states that can be generated using passive linear optics alone is fundamentally constrained by bosonic symmetries. Heralding, based on conditional measurements on auxiliary modes, is a widely used technique to overcome these limitations and effectively enlarge the set of accessible states. Despite the widespread use of heralding, it is often unclear how specific ancillary resources impact the overall reachability of the target space. In this work, we investigate the local controllability of photonic states in linear optical networks by analyzing the rank of the Jacobian of the output state with respect to the underlying unitary circuit, which provides a quantitative measure of the dimension of the accessible tangent space at a given configuration. Our analysis ranges from passive linear optics to heralded linear optics, where auxiliary resources and conditional measurements are included. Within this framework, we quantify how different resources enlarge the locally accessible state space beyond that of passive linear optics and determine the resources required for the Jacobian rank to reach its maximal value, thereby achieving full local controllability. As maximal local rank is a necessary condition for global reachability, our framework offers a systematic tool to assess and compare the accessible state space of measurement-based photonic architectures, and to establish practical criteria for the resources needed in high-dimensional quantum state engineering.
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Enhancing the controllability of quantum systems via a static field
Abstract
We provide a sufficient condition for the controllability of a bilinear closed quantum system steered by a static field and a time-varying field, based on the notion of weakly conically connected spectrum. More precisely, we show that if a controlled Hamiltonian with two inputs has a weakly conically connected spectrum, then, freezing one of the two inputs at almost every constant value, the obtained single-input system is controllable. The result is illustrated with two examples, enantio-selective excitation in a chiral molecule and the driven Jaynes-Cummings Hamiltonian.
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Quantum control of ro-vibrational dynamics and application to light-induced molecular chirality
Abstract
Achiral molecules can be made temporarily chiral by excitation with electric fields, in the sense that an average over molecular orientations displays a net chiral signal [Tikhonov et al., Sci. Adv. 8, eade0311 (2022)]. Here, we go beyond the assumption of molecular orientations to remain fixed during the excitation process. Treating both rotations and vibrations quantum mechanically, we identify conditions for the creation of chiral vibrational wavepackets -- with net chiral signals -- in ensembles of achiral molecules which are initially randomly oriented. Based on the analysis of symmetry and controllability, we derive excitation schemes for the creation of chiral wavepackets using a combination of (a) microwave and IR pulses and (b) a static field and a sequence of IR pulses. These protocols leverage quantum rotational dynamics for pump-probe spectroscopy of chiral vibrational dynamics, extending the latter to regions of the electromagnetic spectrum other than the UV.
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Chattering Phenomenon in Quantum Optimal Control
Abstract
We present a quantum optimal control problem which exhibits a chattering phenomenon. This is the first instance of such a process in quantum control. Using the Pontryagin Maximum Principle and a general procedure due to V. F. Borisov and M. I. Zelikin, we characterize the local optimal synthesis, which is then globalized by a suitable numerical algorithm. We illustrate the importance of detecting chattering phenomena because of their impact on the efficiency of numerical optimization procedures.
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Quantum optimal control in quantum technologies. Strategic report on current status, visions and goals for research in Europe
Abstract
Quantum optimal control, a toolbox for devising and implementing the shapes of external fields that accomplish given tasks in the operation of a quantum device in the best way possible, has evolved into one of the cornerstones for enabling quantum technologies. The last few years have seen a rapid evolution and expansion of the field. We review here recent progress in our understanding of the controllability of open quantum systems and in the development and application of quantum control techniques to quantum technologies. We also address key challenges and sketch a roadmap for future developments.
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Introduction to the Pontryagin Maximum Principle for Quantum Optimal Control
Abstract
Optimal Control Theory is a powerful mathematical tool, which has known a rapid development since the 1950s, mainly for engineering applications. More recently, it has become a widely used method to improve process performance in quantum technologies by means of highly efficient control of quantum dynamics. This tutorial aims at providing an introduction to key concepts of optimal control theory which is accessible to physicists and engineers working in quantum control or in related fields. The different mathematical results are introduced intuitively, before being rigorously stated. This tutorial describes modern aspects of optimal control theory, with a particular focus on the Pontryagin Maximum Principle, which is the main tool for determining open-loop control laws without experimental feedback. The different steps to solve an optimal control problem are discussed, before moving on to more advanced topics such as the existence of optimal solutions or the definition of the different types of extremals, namely normal, abnormal, and singular. The tutorial covers various quantum control issues and describes their mathematical formulation suitable for optimal control. The connection between the Pontryagin Maximum Principle and gradient-based optimization algorithms used for high-dimensional quantum systems is described. The optimal solution of different low-dimensional quantum systems is presented in detail, illustrating how the mathematical tools are applied in a practical way.
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Complete Controllability Despite Degeneracy: Quantum Control of Enantiomer-Specific State Transfer in Chiral Molecules
Abstract
We prove complete controllability for rotational states of an asymmetric top molecule belonging to degenerate values of the orientational quantum number M. Based on this insight, we construct a pulse sequence that energetically separates population initially distributed over degenerate M-states, as a precursor for orientational purification. Introducing the concept of enantio-selective controllability, we determine the conditions for complete enantiomer-specific population transfer in chiral molecules and construct pulse sequences realizing this transfer for population initially distributed over degenerate M-states. This degeneracy presently limits enantiomer-selectivity for any initial state except the rotational ground state. Our work thus shows how to overcome an important obstacle towards separating, with electric fields only, left-handed from right-handed molecules in a racemic mixture.
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Effective adiabatic control of a decoupled Hamiltonian obtained by rotating wave approximation
Abstract
In this paper we study up to which extent we can apply adiabatic control strategies to a quantum control model obtained by rotating wave approximation. In particular, we show that, under suitable assumptions on the asymptotic regime between the parameters characterizing the rotating wave and the adiabatic approximations, the induced flow converges to the one obtained by considering the two approximations separately and by combining them formally in cascade. As a consequence, we propose explicit control laws which can be used to induce desired populations transfers, robustly with respect to parameter dispersions in the controlled Hamiltonian.
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Ensemble qubit controllability with a single control via adiabatic and rotating wave approximations
Abstract
In the physics literature it is common to see the rotating wave approximation andthe adiabatic approximation used "in cascade" to justify the use of chirped pulses for two-level quantum systems driven by one external field, in particular when the resonance frequency of the system is not known precisely. Both approximations need relatively long time and are essentially based on averaging theory of dynamical systems. Unfortunately, the two approximations cannot be done independently since, in a sense, the two time scales interact. The purpose of this paper is to study how the cascade of the two approximations can be justified and how large becomes the final time as the fidelity goes to one, while preserving the robustness of the adiabatic strategy. Our first result, based on high-order averaging techniques, gives a precise quantification of the uncertainty interval of the resonance frequency for which the population inversion works. As a byproduct of this result, we prove that it is possible to control an ensemble of spin systems by a single real-valued control, providing a non-trivial extension of a celebrated result of ensemble controllability with two controls by Khaneja and Li.
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An obstruction to small-time controllability of the bilinear Schr{ö}dinger equation
Abstract
In this article we discuss which controllability properties of classical Hamiltonian systems are preserved after quantization. We discuss some necessary and some sufficient conditions for small-time controllability of classical systems and quantum systems using the WKB method. In particular, we investigate the conjecture that if the classical system is not small-time controllable, then the corresponding quantum system is not small-time controllable either.